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Indeed they are old. Both items and also a long pair of earrings belonged to inheritance princess Caroline. They were bought by the then crown princess Lovisa at the auction following Caroline's death in 1881.
Not worn often but on rare occasions. Pict. 5 can be devided into two pieces. Worn at the state visit in England. And also at the incoming visit from Holland.
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I love the brooches at 2 and 5, they look like old pieces, never saw them worn before though by any of the Danish royals.