Worthy picks at the top two, but I have to say "I Am A Scientist" has never done much for me.
Glad to see "Subspace Biographies" and "Death of the Party", two of the few non-GBV Pollard songs I know well.
My offhand top 20 or so, in roughly chronological order:
Lips of Steel
Under the Neptune/Mesh Gear Fox
Exit Flagger
Goldheart Mountaintop Queen Directory
Tractor Rape Chain
Echos Myron
Blimps Go 90
As We Go Up, We Go Down
Closer You Are
Drag Days
Sad If I Lost It
Jane of the Waking Universe
Teenage FBI
Chasing Heather Crazy
Hold On Hope
The Best of Jill Hives
Subspace Biographies
Heaven Beats Iowa
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